Sarah - if you entered into a Deed of Trust and then a Deed of surrender then we'd need that plus RX3 and ST5 - see our
online guidance
You may find you don;t need to do a second deed though if you are in essence 'tearing the deed of trust up' but much may depend on how it's worded with regards how it might be ended for example.
We can't really advise you on what's needed as the key will be the original Deed and intention - if you need a second deed to end the arrangement then that's worth considering
We won't consider the application until you lodge it so it might be worth having a chat with whoever created the deed for you or with a new legal adviser as appropriate just to be sure