Hello Thomas - a noted rentcharge can be removed on application in
form CN1 along with supporting evidence to show how it has determined (come to an end) and confirming it can be removed from the register
As you already appreciate it will be the supporting evidence that matters here and that's where your legal advice must come in. If you are relying on adverse possession of the rentcharge due to for example non-payment for a period of time then your legal advice should focus on the legislation you refer to. Any supporting evidence would then rely on the facts as to how possession of the rentcharge has then been taken from the rentcharge owner.
We can't advise you on the legal requirements